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Trace Elemental Analysis of Drugs of Abuse Using Synchrotron Radiation Total Reflection X-Ray Fluorescence Analysis (SR-TXRF)

NCJ Number
197317
Journal
Journal of Forensic Sciences Volume: 47 Issue: 5 Dated: September 2002 Pages: 944-949
Author(s)
Seiji Muratsu M.S.; Toshio Ninomiya Ph.D.; Yasushi Kagoshima Ph.D.; Junji Matsui Ph.D.
Date Published
September 2002
Length
6 pages
Annotation
This paper reports on the use of synchrotron radiation total reflection X-ray fluorescence spectroscopy (SR-TXRF) to analyze various trace elements in small amounts of drugs of abuse.
Abstract
Sample amounts of 1 ml solutions that contained 10 pg of drugs (methamphetamine, amphetamine, 3,4-methylene-diosymethamphetamine, cocaine, and heroin) were spotted on silicon wafers for direct analysis. In addition, a leaflet of marijuana was set directly on a silicon wafer; and opium in the form of a soft lump was smeared on another silicon wafer for analysis. The experiments found that 10 pg of contaminant elements could be detected. In a seized methamphetamine sample, iodine was found, which could be indicative of synthetic route. In seized 3,4-methylenedioxymethamphetamine samples, variable amounts of phosphorous, calcium, sulfur, and potassium were found, which could not be detected in a control 3,4-methylenedioxymethamphetamine sample. For marijuana and opium, two spectral patterns were obtained; they were very different from one another and could be easily distinguished. Thus, using SR-TXRF permits the detection of pg amounts of each trace element in 10 mg of various drugs. This is not the case for either a standard TXRF experimental system or for other elemental analysis techniques. 7 illustrative figures and 33 references